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二甲基二氢化芘
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     2)The introduction and translation of T.
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The magnetic coupling of a diarylethene with two nitronyl nitroxide compounds, which exhibits excellent photoswitching performance, was investigated by means of the density functional theory combined with broken-symmetry approach (DFT-BS) method. The calculated results verify that the magnetic coupling is changed with opening and closure of the ring. The same method was used to study model molecules of dimethyl dihydro pyrene with two nitronyl nitroxides. It was also found that the magnetic behavior of the open...

The magnetic coupling of a diarylethene with two nitronyl nitroxide compounds, which exhibits excellent photoswitching performance, was investigated by means of the density functional theory combined with broken-symmetry approach (DFT-BS) method. The calculated results verify that the magnetic coupling is changed with opening and closure of the ring. The same method was used to study model molecules of dimethyl dihydro pyrene with two nitronyl nitroxides. It was also found that the magnetic behavior of the open structures is different from that of close structure for the model molecules, hence the designed model molecules may also have the photoswitching performance.

采用密度泛函结合对称性破损态(DFT-BS)方法,通过计算具有光控磁性分子开关功能的二氮氧自由基二芳基乙烯化合物的磁偶合常数,合理解释了其分子结构发生开环和闭环变化时,分子磁性发生的改变.同时设计了二氮氧自由基二甲基二氢化芘分子光控开环和闭环模型,并用同样的方法计算了模型分子的磁偶合常数,发现这些模型分子的磁行为类似于二氮氧自由基二芳基乙烯化合物,有可能也具有光控磁性分子开关功能.

 
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