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The structure and property of the high resolution α-γ coincidence spectrometer and its; applications in determining heavy nuclide qualitatively and quantitatively are described. At present, the energy resolution of the spectrometer is 0.25% (for 5.486MeV aaaaaaaaa particle,, FWHM is 13.8keV); the energy shift of peak is 0.05% during eight hours; nonlinearity is less than 0.2% for the energy region from 4 to 8 MeV.The α probe of the spectrometer mainly consists of a silicon-gold surface barrier detector... The structure and property of the high resolution α-γ coincidence spectrometer and its; applications in determining heavy nuclide qualitatively and quantitatively are described. At present, the energy resolution of the spectrometer is 0.25% (for 5.486MeV aaaaaaaaa particle,, FWHM is 13.8keV); the energy shift of peak is 0.05% during eight hours; nonlinearity is less than 0.2% for the energy region from 4 to 8 MeV.The α probe of the spectrometer mainly consists of a silicon-gold surface barrier detector with active area 50 mm2 or 314 mm2. The detector is cooled by thermoelectric technique with a low-power Peltier element. Its temperature is decreased form room tem-perature (25℃) to - 25℃. Thus its leakage-current is decresed by 2 orders of magnitude and the system noise is also decreased; the energy resolution of the spectrometer is thus-raised.A 40×35 mm well type Nal (T1) scintillation crystal with 20 mm in well diameter and 25mm in well depth is employed in the γ probe of the spectrometer. The well wall of crystal is covered with 0.5mm thick aluminium. The crystal active thickness is about. 10mm. Thus both the loss of low energy γ-rays and the background of high energy γ-rays are decreased. At the same time, the nuclide measurement sensitivity and accuracy of mixture source are raised by changing source position to be measured in the well.In this paper, the method is being applied to the determination of 241Am in the presence of large amount of Cm and fission products, for example, when the ratio of241Am/242Cm equals 2×10-5 (α activity). It is convenient and accurate to measure 238Pu and 241Am in which the ratio of a activity is in the region of 10-2-50. Besides, it can be applied to the absolute measurement of transplutonium nuclides. Its accuracy is better than±1%. 本文描述了高分辨率α-γ符合谱仪的结构、性能指标及其在重元素核素的相对和绝对含量测定中的应用。目前该谱仪的符合α能谱的能量分辨率为0.25%(对5.486兆电子伏,FWHM=13.8千电子伏);稳定性在八小时内能峰漂移为±0.05%;4—8兆电子伏区间能量非线性<0.2%。文中还简略地叙述了一些实际应用的测量原理及其方法。 The absolute intensity of medical isotopes 181I and 198Au with a short half-life has been measured by the efficiency extrapolation method of Aπβ-γ coincidence absorption curve. The result of the measurement has been corrected for background, dead time, resolving time respectively. The correction for the short half-life has also been considered. The maximum error of the measurement are 0.57% and 1.7% for 131I and 198Au respectively. After a little change of the apparatus, we have measured the nuclide with... The absolute intensity of medical isotopes 181I and 198Au with a short half-life has been measured by the efficiency extrapolation method of Aπβ-γ coincidence absorption curve. The result of the measurement has been corrected for background, dead time, resolving time respectively. The correction for the short half-life has also been considered. The maximum error of the measurement are 0.57% and 1.7% for 131I and 198Au respectively. After a little change of the apparatus, we have measured the nuclide with electron capture decay. 用4πβ-γ符合吸收曲线效率外推法,测定短寿命的医用同位素~(131)I、~(198)Au绝对强度。测量结果分别对本底、死时间、分辨时间进行了修正,同时还考虑了短半衰期引起的修正。对~(131)I和~(198)Au的最大测量误差分别为0.57%和1.7%。本装置稍作改变后,还测量了具有电子俘获衰变的核素。 In the experiments 610 rats,some guinea pigs,rabbits anddogs were used to study the therapeutic effect of the Tiron,a kind of che- late,on removing uranium from the poisoned animals received lethal doseof uranyl nitrate.The results showed that the Tiron is significantly superiorto the EDTA and DTPA in removing nuclide from the animals body and isable to reduce the mortality of poisoned animals.in the control groupswithout chelate treatment,90—100% of the poisoned animals died of uran-ium poisoning within... In the experiments 610 rats,some guinea pigs,rabbits anddogs were used to study the therapeutic effect of the Tiron,a kind of che- late,on removing uranium from the poisoned animals received lethal doseof uranyl nitrate.The results showed that the Tiron is significantly superiorto the EDTA and DTPA in removing nuclide from the animals body and isable to reduce the mortality of poisoned animals.in the control groupswithout chelate treatment,90—100% of the poisoned animals died of uran-ium poisoning within 30 days;but in the treated groups with Tiron,90—100% of the animals have been living throughout all experimental period.The uranium content in the excreted urine of those animals treated withTiron was 2—3 times more than that of the control.But delayed treatmentwith Tiron at 24 hours after administration of nuclide was not so effectiveas the early treatment.The toxicity of the Tiron to the kidney is lower thanthat of EDTA and DTPA.The Tiron's LD_(50)is about 6.0 grams per 1 kgbody weight in mice and in rats. 本实验用了610只大鼠、少量豚鼠、家兔和狗,研究了 Tiron 这种螯合剂对接受致死剂量硝酸铀酰中毒动物的排铀治疗效果。实验结果表明,Tiron 在促排核素和降低死亡率上明显地优于EDTA 和 DTPA。在对照组中,90—100%的动物在30天内因铀中毒而死亡;但用 Tiron 治疗的动物中,90—100%的动物都能在实验期内活存下来。给与 Tiron 的动物,其尿铀排出量比对照组多1—2倍。但若在注射核素后24小时给与 Tiron 时,不如早期给药那么有效。Tiron 对肾的毒性比 EDTA 和 DTPA 都低,对小鼠和大鼠的 LD_(SO)为6克每公斤体重左右。
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