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Magnetization curves of the polycrystalline Fe-Co and Ni-Co alloys of the cubic system and also of the pure cobalt were determined by means of a ballistic method. Gans' theory of the magnetic properties of isotropic ferromagnetics was applied. The agreement between his theory and the experimental results is quite good for the strong fields but not so for the weak fields, just as in the ease of the pure ferromagnetics. The discrepancy for the weak fields may be explained by his neglect of the free energy which...

Magnetization curves of the polycrystalline Fe-Co and Ni-Co alloys of the cubic system and also of the pure cobalt were determined by means of a ballistic method. Gans' theory of the magnetic properties of isotropic ferromagnetics was applied. The agreement between his theory and the experimental results is quite good for the strong fields but not so for the weak fields, just as in the ease of the pure ferromagnetics. The discrepancy for the weak fields may be explained by his neglect of the free energy which is required to magnetize the elementary crystals isothermally to the saturation intensities in the easy direction of magnetization. After including this part of the energy the agreement between theory and experiment is improved in general and in some cases, it is remarkably good. For pure cobalt the magnetization intensities for a given field are smaller than those obtained by previous investigators, but in better agreement with the theory than those previously obtained. Since the disagreement cannot be accounted for by the experimental error in the present investigation, the comparatively less studied cobalt needs further investigation.

用冲击法量属於正方晶系之铁钴及镍钴合金并纯钴之多结晶体之磁化曲线与Gans氏各向同性铁磁物质磁性之理论相较知在强磁场时理论与实验之契合甚佳在弱磁场时则较差,弱磁场时之差异,可以Gans氏计算时略去磁化各晶体於其易磁化方向至饱和度所需之自由能一点解释之改正此点后理论与实验之契合大体改善在数种合金且极佳。纯钴之磁化强度在各磁场下较之前人所得者均小,惟与理论之契合则较佳:此与前人不同之点既不能归诸本实验之误差,则此较少被注意之钴实需要更进一步之研究

In the statistical theory of superlattices in binary alloys, the dependence of the interaction energy upon atomic arrangements is taken into account by regarding the interaction energy in Bethe's theory as an average quantity depending on the degree of order and the composition of the alloy. Two simple assumptions concerning the functional relationship of the interaction energy with order and composition are made. The first is a linear function of order and composition. The second is a linear function of the...

In the statistical theory of superlattices in binary alloys, the dependence of the interaction energy upon atomic arrangements is taken into account by regarding the interaction energy in Bethe's theory as an average quantity depending on the degree of order and the composition of the alloy. Two simple assumptions concerning the functional relationship of the interaction energy with order and composition are made. The first is a linear function of order and composition. The second is a linear function of the average numbers of pairs of atoms. The result of applying these assumptions to superlattices of the type AB is that the critical temperature as a function of the composition is a maximum for equal sumber of A and B atoms only when a certain relation between the coefficients in the assumed function is satisfied. In the cass of superlattices of type AB3 the theory of Bragg and Williams is used for simplicity. It is shown that when the composition varies, the maximum of the critical temperature may occur at any desired composition by a suitables adjustment of the coefficients in the assumed functions. There is thus a hope of removing the discrepancy between theory and experiment on this line. The anomalous specific heat at the critical temperature is also calculated for different compositions. In the case of the AB type of superlattices, Bethe's formula for the energy is no longer valid, and in order to calculate the specific heat, an approximate formula for the energy is obtained by analogy with the theory of Bragg and Williams. Finally, the problem of separation into more than one phase is briefly discussed.

在二合金超格之统计力学理论中,原子间互作用能量,因原子之排列不同而异,其所生之影响,吾人擬於此篇中讨论之。吾人认为有Bethe氏理论中之相互作用能量,实为一平均值,其值因合金之秩序程度及其成分而异。吾人作二简单假设:一设相互作用能量为秩序及成分之线性函数,另一设其与原子对偶之数成线性函数。将此等假设应用於AB类之合金,则必须在所设函数中之系数间,有适当关系,合金之临界温度,始在成分为1:1时,有极大值。在AB_3类之合金,吾人乃应用Bragg及Williams二氏之理论以求简便。於此可证明若所设函数中之系数,可任意调整则所计算出之临界温度之极大值可在任何成分发生。故关於此点理论与实验不合之处,可望解决。又合金之反常比热,亦经算出。在AB类之合金,Bethe氏原来之能量公式不復可用,故另用与Bragg及Williams理论比较而得之公式计算。又关於合金可分为二相或多相之问题,此篇亦大略论及。

General formulas for the. critical temperature and the discontinuity of the ipecific heat of a, superlattice are obtained by the generalized quasi-chemical method, The results may be applied to any approximation.

本文应用推广准化学方法求得二超格结晶在任何几近计算中之临界温度及比热突变公式。

 
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